10.3. SCALE Nuclear Data Covariance Library

A. Holcomb, D. Wiarda, M. L. Williams, G. Arbanas, and B. L. Broadhead

ABSTRACT

An updated cross section covariance library has been created for use with the sensitivity and uncertainty modules in SCALE 6.3. The data have been assembled from a variety sources, including high-fidelity covariance evaluations from ENDF/B-VIII.0 as well as approximate uncertainties obtained from a collaborative project performed by Brookhaven National Laboratory, Los Alamos National Laboratory, and Oak Ridge National Laboratory. This document describes the assumptions in generating the data, the library contents, and processing procedure for the SCALE 56-group and 252-group covariance libraries. The ENDF/B-VII.1 covariance libraries provided with SCALE 6.3 are identical to the libraries released with SCALE 6.2. The SCALE 44-group covariance library distributed with SCALE 6.0 and SCALE 6.1 is retained for backwards compatibility.

ACKNOWLEDGMENT

We gratefully acknowledge the sponsorship of the US Department of Energy Nuclear Criticality Safety Program in the development of the SCALE 6.3 covariance libraries.

10.3.1. Introduction

The SCALE 6.3 covariance library suite contains covariance libraries based on ENDF/B-VIII.0, ENDF/B-VII.1, and pre-ENDF/B-VII.0. For each ENDF release, if uncertainty information is not available for all neutron targets, then the corresponding SCALE covariance library is patched such that each library has some estimate of the uncertainty data for every neutron target in the library. The ENDF/B-VIII.0 covariance library [XSLibDAB18] contains at least some covariance data for 252 nuclides and the ENDF/B-VII.1 library [COVLIBCHO+11] has data for 187 nuclides. Both the ENDF/B-VIII.0 and ENDF/B-VII.1 covariance libraries have been supplemented by the previous SCALE 6.1 covariance data for the ~305 nuclides missing covariance data in ENDF/B-VIII.0 and ~215 nuclides missing covariance data in ENDF/B-VII.1. The ENDF/B-VII.1 uncertainties were modified for a few nuclides, as described in Sect. 10.3.2.3. The ENDF/B-VIII.0 covariance data are available in a 56-group format, and the ENDF/B-VII.1 covariance library is in both a 56-group and 252-group format. These covariance libraries were generated for compatibility with the ENDF/B-VII.1 cross section libraries distributed with SCALE 6.3, and they may also be applied for the 238-group ENDF/B-VII.0 library provided with SCALE 6.2. The previous SCALE 6.0 and SCALE 6.1 44-group library (44groupcov) was based on older covariance data and is retained in SCALE 6.3 for backwards compatibility. However, the 56- and 252-group covariance libraries (56groupcov7.1 and 252groupcov7.1) are now recommended for all applications. The 56-group library-which is default for SCALE uncertainty analysis-and the 252 fine-group library generally produce similar results, except for some threshold reactions such as (n,2n). The 252-group library may be used to improve uncertainty estimates from these types of data, but it takes more execution time than the default 56-group library. Because the 56- and 252-group covariance data in many cases are based on newer uncertainty evaluations than the previous 44-group library, some differences will occur between these sets of results.

The covariance data correspond to relative uncertainties assembled from a variety of sources, including evaluations from ENDF/B-VIII.0, ENDF/B-VII.1, ENDF/B-VI, and approximated uncertainties from a collaborative project performed by Brookhaven National Laboratory (BNL), Los Alamos National Laboratory (LANL), and Oak Ridge National Laboratory (ORNL). Because SCALE uncertainty data come from several different sources, the application of a single generic covariance library to all multigroup cross section libraries raises questions about consistency with any given data evaluation. In reality, much of the approximate uncertainty data in the library is based on simplifying approximations that do not depend on specific ENDF evaluations and thus can be applied to all cross section libraries within the limitations of the assumed methodology. In other cases in which a covariance evaluation has been taken from a specific nuclear data file (e.g., ENDF/B-VIII.-,ENDF/B-VII.1, ENDF/B-VI, or JENDL), it is assumed that the same relative (rather than absolute) uncertainties can be applied to all cross section libraries, even if these are not strictly consistent with the nuclear data evaluations. The assumption is partially justified by the fact that different evaluations often use many of the same experimental measurements since there is a limited amount of this information available. In some cases, older data evaluations have been carried over into the newer ENDF versions. Also, because many important nuclear data are now known rather well, newer evaluations in many instances correspond to rather modest variations from previous ones and are expected to lie within the earlier uncertainties.

No inherently “true” uncertainty can be defined for nuclear data. For example, in theory, two independent evaluations could produce similar nuclear data with very different uncertainties. Differences in nuclear data evaluations directly impact calculations that can be affirmed by comparisons with benchmark experiments; but there is no established procedure to quantify the reliability of uncertainty estimates. In general, the SCALE covariance library should be viewed as a best-estimate assessment of data uncertainties based upon the specific methodology described in the following section. While this methodology is not unique and other approaches could have been used, the SCALE covariance library is a reasonable representation of the nuclear data uncertainties for most applications given the current lack of information. Furthermore, it is the only available comprehensive library that has been created in a well-defined, systematic manner.

10.3.2. Covariance Data Description

10.3.2.1. Evaluated covariances from nuclear data files

A rigorous, modern evaluation of nuclear data typically uses a regression algorithm that adjusts parameters in a nuclear physics model (e.g., Reich-Moore resonance formula, optical model, etc.), to fit a set of differential experimental measurements that have various sources of statistical and systematic uncertainties [COVLIBLLD+06]. Information from the regression analysis of the model parameters can be propagated to uncertainties and correlations in the evaluated differential data. In this manner, the differential nuclear data and covariances are consistent and are coupled together by evaluation processes. Unfortunately, only a limited number of cross section evaluations have produced high-fidelity covariances in this rigorous manner. All other nuclear data uncertainties must be estimated from approximations in which the uncertainty assessment is decoupled from the original evaluation procedure.

The SCALE covariance library is based on several different uncertainty approximations with varying degrees of fidelity relative to the actual nuclear data evaluation. The library includes high-fidelity evaluated covariances obtained from the latest ENDF releases whenever available. As discussed in Sect. 10.3.1, it is assumed that covariances taken from one data evaluation, such as ENDF/B-VII.1, can also be applied to other evaluations of the same data, such as ENDF/B-VIII.0. If this is done judiciously for cases in which the nuclear data evaluations are similar, then the covariances taken from one source should be a reasonable representation of uncertainties for the other evaluations.

10.3.2.2. Approximate covariance data

At the other end of the spectrum from high fidelity data, low-fidelity (lo-fi) covariances are defined to be those estimated independently of a specific data evaluation. The approximate covariance data in SCALE are based on results from a collaborative project funded by the US Department of Energy Nuclear Criticality Safety Program to generate lo-fi covariances over the energy range from 10-5 eV to 20 MeV for materials without covariances in ENDF/B-VII.1. Nuclear data experts at BNL, LANL, and ORNL devised simple procedures to estimate data uncertainties in the absence of high fidelity covariance evaluations. The result of this project is a set of covariance data in ENDF/B file 33 format that can be processed into multigroup covariances [COVLIBLKH+08]. Some of these data were later revised and included in ENDF/B-VII.1, while others were carried over from SCALE 6.1 to the SCALE 6.3 library. In this documentation, these data are known as BLO (BNL-LANL-ORNL) uncertainty data, which were generated as described below.

ORNL used uncertainties in integral experiment measurements of thermal cross sections, resonance integrals, and potential cross sections to approximate the standard deviations of capture, fission, and elastic scattering reactions for the thermal (<0.5 eV) and resonance ranges (0.5 eV- 5 keV). Full energy correlation was assumed for the covariances within each of these respective ranges [COVLIBWBDR07, COVLIBWR08] This procedure was originally introduced for the approximate uncertainty data in SCALE 5.1. However, the current version includes updated integral measurement uncertainties, using the more recent values tabulated by Mughabghab in the Atlas of Neutron Resonances [COVLIBMug06]. The lo-fi relative uncertainty is computed as the absolute uncertainty in the integral parameter (i.e., thermal cross section or resonance integral) taken from the Atlas, divided by the average of the measured parameter and the calculated value computed from ENDF/B-VII differential data:

(10.3.1)\[\mathrm{U}=\frac{\Delta_{\mathrm{I}}}{0.5 \times\left(\mathrm{X}_{\mathrm{I}}+\mathrm{X}_{\mathrm{D}}\right)} ,\]

where:

U is the relative lo-fi uncertainty included in SCALE,

\(\Delta\)I is the absolute uncertainty in the integral measurement (obtained from Mughabghab), and

XI and XD are the measured and computed (from ENDF/B differential data) integral parameter values, respectively.

In some cases the integral measurement value from the Mughabghab Atlas6 and the corresponding value computed from the ENDF/B-VII differential evaluation are inconsistent-defined here as having a difference greater than two standard deviations in the measured and computed integral parameters. In these cases, the lo-fi relative standard deviation is defined as half the difference relative to the average of the measured and calculated values:

(10.3.2)\[\mathrm{U}=\frac{\left|\mathrm{X}_{\mathrm{I}}-\mathrm{X}_{\mathrm{D}}\right|}{\mathrm{X}_{\mathrm{I}}+\mathrm{X}_{\mathrm{D}}} ; \text { for }\left|\mathrm{X}_{\mathrm{I}}-\mathrm{X}_{\mathrm{D}}\right|>2 \Delta_{\mathrm{I}} .\]

In some instances this expression may exceed 100%. For these cases, a 100% uncertainty was assigned. Also, the Atlas does not include uncertainties in integral measurements for several isotopes, which typically are not of great interest for most applications. In this case the integral uncertainty was defined as a +/-5 in the least significant digit for these materials; e.g., 1.23 is assign an uncertainty of +/- 5E-3.

BNL and LANL provided estimates in the fast energy range from 5 keV to 20 MeV for covariances of capture, fission, elastic, inelastic, (n,2n) cross sections, and prompt nubar. BNL used optical model calculations with estimated uncertainties in model parameters to compute covariances in the fast range for about 300 structural isotopes, fission products, and non-fissionable heavy nuclei. Estimated uncertainties in model parameters were based on previous work and expert judgment [COVLIBPHO09]. Covariances for 14 actinide isotopes were obtained from earlier work performed by BNL for Subgroup-26 (SG-26) [COVLIBRHOM07]. The SG-26 actinide covariances cover the full energy range, including thermal, resonance, and fast regions. If the thermal data uncertainties estimated by the SG-26 approach exceed the thermal uncertainty given in reference 6, the thermal data covariances are represented by ORNL’s integral uncertainty technique.

LANL produced covariances in the fast range for an additional 47 actinide materials. The LANL actinide covariances were based on empirical estimates of nuclear reaction models [COVLIBKTY+08]. Full energy range covariances were also produced by LANL for 16 light isotopes ranging from hydrogen to fluorine [COVLIBHal08]. These included high fidelity covariances from R-matrix analyses for 1H, 6Li, and 10B, along with lo-fi uncertainties for the other materials, based on approximations such as least-squares fitting to experimental data, statistical model calculations at higher energies, or sometimes simply best-judgment estimation [COVLIBLKH+08].

10.3.2.3. Modifications to covariance data

In generating earlier covariance libraries, some omissions or inconsistencies were identified and corrected in the current covariance library:

  • If the absolute correlation is larger than 1, it is set to 1.

  • If a relative uncertainty is larger than 1, it is set to 1.

  • If cross section data exist but covariance data do not span the entire range, then the diagonal element for the higher energy groups is repeated for the lower energy groups.

  • If total inelastic scattering covariance is not supplied, it is calculated from the uncertainties in the discrete level inelastic data.

  • If total nubar covariance is not supplied, it is calculated from the the prompt and delayed nubar uncertainties

A few inconsistencies were found in the ENDF/B-VII.1 uncertainty data, and these were modified for the SCALE 6.3 covariance library [COVLIBWIMR14]. The corrections were also conveyed to the National Nuclear Data Center, where they were added to the ENDF/A file for possible inclusion in the future release of ENDF/B-VIII.1. These modifications are summarized below:

  1. 235U thermal nubar: standard deviation was decreased from 0.7% to 0.3% in energy range from 0.0 to 0.5 eV, consistent with JENDL-3.3.

  2. 239Pu thermal nubar: standard deviation was increased from 0.01% to 0.15% in energy range from 0.0 to 0.01 eV, consistent with ENDF/B-VII.1 uncertainty at 0.01 eV.

  3. H thermal capture: standard deviation reduced from 2.5% to 0.2%, consistent with Williams and Rearden 2008 [COVLIBWR08],

(d) 103Rh thermal capture: reduced from ~4% to 1.04%, consistent with Williams and Rearden 2008 [COVLIBWR08].

(e) 151Sm thermal capture: modified to ~1.8%, consistent with Williams and Rearden 2008 [COVLIBWR08].

(f) 147Pm: standard deviation was reduced from 24% to 5% in the energy range 0.5–5000 eV, consistent with the quoted resonance integral uncertainty in Williams and Rearden 2008 [COVLIBWR08].

Several modifications were also made to the uncertainties obtained from the original BLO data used in SCALE 6.1. The energy boundary between the thermal and resonance covariance blocks was modified from 0.5 to 0.625 eV in order to coincide with a 56-group boundary. The BLO lo-fi data do not include thermal or resonance range uncertainties for isotope reactions that do not have integral uncertainties given in the Mughabghab text [COVLIBMug06]. These occur mainly for relatively unimportant data such as elastic cross sections of several fission products. Therefore in these cases the uncertainties were estimated using different approaches. For example, the thermal data uncertainty was sometimes used to represent the epithermal uncertainty if it was not available in the Mughabghab tabulation, and sometimes the high-energy uncertainty was extended to lower energies. The uncertainty in the 149Sm resonance capture integral is not provided in the 2006 edition of Mughabghab’s text, so it was set to the value of 5.7%, which was obtained from an earlier tabulation by Mughabghab [COVLIBMug03].

10.3.2.4. Covariance data for fission spectra

As of ENDF/B-VII.1, covariance matrices are now provided for the fission exit energy distribution. The data are given as a function of incident energy. The incident energy grid is very broad, and the exit energy distribution is constant over a given incident energy group. Since the COVERX library file only allows one multigroup fission spectrum (\(\chi\)) covariance matrix per nuclide, the exit energy spectrum is used for the average energy of fission. If \(\nu\) is nubar, f is fission, and w is the appropriate flux, then the average energy of fission is calculated as:

(10.3.3)\[10^{7} \exp \left(-\frac{\sum v f w \frac{1}{2}\left(\log \left(\frac{10^{7}}{E_{g 1}}\right)+\log \left(\frac{10^{7}}{E_{g 2}}\right)\right)}{\sum v f w}\right)\]

where the sum is over all groups and Eg1 and Eg2 are the group boundaries for group g. ENDF/B-VII.1 provides covariance data for exit energy distributions for 64 nuclides. This includes all nuclides for which fission spectrum (\(\chi\)) covariance matrices where provided in the previous covariance library. Some additional \(\chi\)-covariance matrices were taken from JENDL-4.0. The new 56-group and 252-group fission spectrum covariances are more complete and significantly improved compared to the earlier 44-group chi uncertainty data, which were based on the Watt fission spectrum in ENDF/B-V. (see Sect. 10.3.5).

10.3.3. Multigroup Covariance Processing

Covariance data were processed with the AMPX code PUFF-IV [COVLIBWD06]. PUFF-IV has major improvements in the treatment of the resolved and unresolved resonance parameter uncertainties over previous code versions [COVLIBWALD08]. All nuclides with resonance parameter uncertainty files were processed with the full sensitivity option in PUFF-IV.

10.3.4. Contents of the SCALE 6.3 Covariance Library

The SCALE covariance library provides uncertainty data in 56- and 252-group formats for a total of 456 materials in ENDF/B-VII.1 and 587 materials in ENDF/B-VIII.0, including some duplication for materials with multiple thermal scattering kernels. Table 10.3.1 describes the contents of the library using the following nomenclature:

  1. ENDF/B-VII.1: evaluated covariance data released with ENDF/B-VII.1

  2. ENDF/B-VII.2-prelim: recently evaluated data proposed for future release of ENDF/B-VII.2

  3. ENDF/B-VI: evaluated covariance data released with ENDF/B-VI

  4. BLO approximate data: lo-fi covariances from BLO project

  5. SG-26: approximate covariances from WPEC Subgroup-26

  6. JENDL-4.0: evaluated covariance data released with JENDL-4.0

Several covariance evaluations include cross correlations between reactions. These are summarized in Table 10.3.2.

Table 10.3.1 Contents of SCALE 6.3 covariance libraries.

SCALE name

SCALE ID

Data source

Comment

ac-225

89225

ENDF/B-VII.1

ac-226

89226

ENDF/B-VII.1

ac-227

89227

ENDF/B-VII.1

ag-107

47107

BLO approximation data

ag-109

47109

ENDF/B-VII.1

ag-110m

1047110

BLO approximation data

ag-111

47111

BLO approximation data

al-27

13027

ENDF/B-VII.1

albound

1013027

ENDF/B-VII.1

Duplicate of al-27

am-240

95240

ENDF/B-VII.1

am-241

95241

ENDF/B-VII.1

\(\chi\) covariance JENDL-4.0

am-242

95242

SG-26

\(\chi\) covariance JENDL-4.0

Thermal uncertainty replaced by Mughabghab value

am-242m

1095242

ENDF/B-VII.1

am-243

95243

ENDF/B-VII.1

\(\chi\) covariance JENDL-4.0

am-244

95244

BLO approximation data

\(\chi\) covariance JENDL-4.0

am-244m

1095244

BLO approximation data

ar-36

18036

BLO approximation data

ar-38

18038

BLO approximation data

ar-40

18040

BLO approximation data

as-74

33074

BLO approximation data

as-75

33075

BLO approximation data

au-197

79197

ENDF/B-VII.1

b-10

5010

ENDF/B-VII.1

b-11

5011

ENDF/B-VII.1

ba-130

56130

BLO approximation data

ba-132

56132

BLO approximation data

ba-133

56133

BLO approximation data

ba-134

56134

BLO approximation data

ba-135

56135

BLO approximation data

ba-136

56136

BLO approximation data

ba-137

56137

BLO approximation data

ba-138

56138

BLO approximation data

ba-140

56140

BLO approximation data

be-7

4007

BLO approximation data

be-9

4009

ENDF/B-VII.1

be-beo

5004009

ENDF/B-VII.1

Duplicate of be-9

bebound

3004009

ENDF/B-VII.1

Duplicate of be-9

bi-209

83209

ENDF/B-VII.1

bk-245

97245

ENDF/B-VII.1

bk-246

97246

ENDF/B-VII.1

bk-247

97247

ENDF/B-VII.1

bk-248

97248

ENDF/B-VII.1

bk-249

97249

ENDF/B-VII.1

bk-250

97250

ENDF/B-VII.1

br-79

35079

BLO approximation data

br-81

35081

BLO approximation data

c

6000

ENDF/B-VII.1

ca

20000

BLO approximation dataca

ca-40

20040

BLO approximation data

ca-42

20042

BLO approximation data

ca-43

20043

BLO approximation data

ca-44

20044

BLO approximation data

ca-46

20046

BLO approximation data

ca-48

20048

BLO approximation data

cd

48000

BLO approximation data

cd-106

48106

BLO approximation data

cd-108

48108

BLO approximation data

cd-110

48110

BLO approximation data

cd-111

48111

BLO approximation data

cd-112

48112

BLO approximation data

cd-113

48113

BLO approximation data

cd-114

48114

BLO approximation data

cd-115m

1048115

BLO approximation data

cd-116

48116

BLO approximation data

ce-136

58136

BLO approximation data

ce-138

58138

BLO approximation data

ce-139

58139

BLO approximation data

ce-140

58140

BLO approximation data

ce-141

58141

ENDF/B-VII.1

ce-142

58142

BLO approximation data

ce-143

58143

BLO approximation data

ce-144

58144

BLO approximation data

cf-246

98246

ENDF/B-VII.1

cf-248

98248

ENDF/B-VII.1

cf-249

98249

ENDF/B-VII.1

cf-250

98250

ENDF/B-VII.1

cf-251

98251

ENDF/B-VII.1

cf-252

98252

ENDF/B-VII.1

cf-253

98253

ENDF/B-VII.1

cf-254

98254

ENDF/B-VII.1

cl

17000

BLO approximation data

cl-35

17035

ENDF/B-VII.1

cl-37

17037

ENDF/B-VII.1

cm-240

96240

ENDF/B-VII.1

cm-241

96241

ENDF/B-VII.1

cm-242

96242

ENDF/B-VII.1

cm-243

96243

ENDF/B-VII.1

cm-244

96244

ENDF/B-VII.1

cm-245

96245

ENDF/B-VII.1

cm-246

96246

ENDF/B-VII.1

cm-247

96247

ENDF/B-VII.1

cm-248

96248

ENDF/B-VII.1

cm-249

96249

ENDF/B-VII.1

cm-250

96250

ENDF/B-VII.1

co-58

27058

BLO approximation data

co-58m

1027058

BLO approximation data

co-59

27059

ENDF/B-VII.1

cr-50

24050

ENDF/B-VII.1

cr-52

24052

ENDF/B-VII.1

cr-53

24053

ENDF/B-VII.1

cr-54

24054

ENDF/B-VII.1

cs-133

55133

ENDF/B-VII.1

cs-134

55134

BLO approximation data

cs-135

55135

ENDF/B-VII.1

cs-136

55136

BLO approximation data

cs-137

55137

BLO approximation data

cu-63

29063

ENDF/B-VI

cu-65

29065

ENDF/B-VI

d

1002

ENDF/B-VII.1

Duplicate of h-2

d-cryo_ortho

4001002

ENDF/B-VII.1

Duplicate of h-2

d-cryo_para

5001002

ENDF/B-VII.1

Duplicate of h-2

dfreegas

8001002

ENDF/B-VII.1

dy-156

66156

BLO approximation data

dy-158

66158

BLO approximation data

dy-160

66160

BLO approximation data

dy-161

66161

BLO approximation data

dy-162

66162

BLO approximation data

dy-163

66163

BLO approximation data

dy-164

66164

BLO approximation data

er-162

68162

BLO approximation data

er-164

68164

BLO approximation data

er-166

68166

ENDF/B-VII.1

er-167

68167

ENDF/B-VII.1

er-168

68168

ENDF/B-VII.1

er-170

68170

ENDF/B-VII.1

es-251

99251

ENDF/B-VII.1

es-252

99252

ENDF/B-VII.1

es-253

99253

ENDF/B-VII.1

es-254

99254

ENDF/B-VII.1

es-254m

1099254

ENDF/B-VII.1

es-255

99255

ENDF/B-VII.1

eu-151

63151

BLO approximation data

eu-152

63152

BLO approximation data

eu-153

63153

ENDF/B-VII.1

eu-154

63154

BLO approximation data

eu-155

63155

ENDF/B-VII.1

Uses ENDF/B-VII.1 data uncertainty in the thermal range for MT=102

eu-156

63156

BLO approximation data

eu-157

63157

BLO approximation data

f-19

9019

ENDF/B-VII.1

fe-54

26054

ENDF/B-VII.1

fe-56

26056

ENDF/B-VII.1

fe-57

26057

ENDF/B-VII.1

fe-58

26058

ENDF/B-VI

febound

1026000

ENDF/B-VII.1

Duplicate of fe-56

fm-255

100255

ENDF/B-VII.1

ga

31000

BLO approximation data

ga-69

31069

BLO approximation data

ga-71

31071

BLO approximation data

gd-152

64152

ENDF/B-VII.1

gd-153

64153

ENDF/B-VII.1

gd-154

64154

ENDF/B-VII.1

gd-155

64155

ENDF/B-VII.1

gd-156

64156

ENDF/B-VII.1

gd-157

64157

ENDF/B-VII.1

gd-158

64158

ENDF/B-VII.1

gd-160

64160

ENDF/B-VII.1

ge-70

32070

BLO approximation data

ge-72

32072

BLO approximation data

ge-73

32073

BLO approximation data

ge-74

32074

BLO approximation data

ge-76

32076

BLO approximation data

graphite

3006000

ENDF/B-VII.1

Duplicate of c

h

1001

ENDF/B-VII.2 prelim

Duplicate of h1

h-3

1003

BLO approximation data

h-benzene

6001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-benzene

5006000

ENDF/B-VII.1

Duplicate of c

h-cryo_ortho

4001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-cryo_para

5001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-liquid_ch4

1001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-poly

9001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-solid_ch4

2001001

ENDF/B-VII.2 prelim

Duplicate of h-1

h-zrh2

7001001

ENDF/B-VII.2 prelim

Duplicate of h-1

he-3

2003

BLO approximation data

he-4

2004

ENDF/B-VII.1

hf

72000

BLO approximation data

hf-174

72174

BLO approximation data

hf-176

72176

BLO approximation data

hf-177

72177

BLO approximation data

hf-178

72178

BLO approximation data

hf-179

72179

BLO approximation data

hf-180

72180

BLO approximation data

hfreegas

8001001

ENDF/B-VII.2 prelim

hg-196

80196

BLO approximation data

hg-198

80198

BLO approximation data

hg-199

80199

BLO approximation data

hg-200

80200

BLO approximation data

hg-201

80201

BLO approximation data

hg-202

80202

BLO approximation data

hg-204

80204

BLO approximation data

ho-165

67165

BLO approximation data

ho-166m

1067166

BLO approximation data

i-127

53127

ENDF/B-VII.1

i-129

53129

ENDF/B-VII.1

i-130

53130

BLO approximation data

i-131

53131

BLO approximation data

i-135

53135

BLO approximation data

in

49000

ENDF/B-VI

in-113

49113

BLO approximation data

in-115

49115

BLO approximation data

ir-191

77191

ENDF/B-VII.1

ir-193

77193

ENDF/B-VII.1

k

19000

BLO approximation data

k-39

19039

ENDF/B-VII.1

k-40

19040

BLO approximation data

k-41

19041

ENDF/B-VII.1

kr-78

36078

BLO approximation data

kr-80

36080

BLO approximation data

kr-82

36082

BLO approximation data

kr-83

36083

BLO approximation data

kr-84

36084

BLO approximation data

kr-85

36085

BLO approximation data

kr-86

36086

BLO approximation data

la-138

57138

BLO approximation data

la-139

57139

ENDF/B-VII.1

la-140

57140

BLO approximation data

li-6

3006

ENDF/B-VII.1

li-7

3007

ENDF/B-VII.1

lu-175

71175

BLO approximation data

lu-176

71176

BLO approximation data

mg

12000

BLO approximation data

mg-24

12024

ENDF/B-VII.1

mg-25

12025

ENDF/B-VII.1

mg-26

12026

ENDF/B-VII.1

mn-55

25055

ENDF/B-VII.1

mo

42000

BLO approximation data

mo-100

42100

ENDF/B-VII.1

mo-92

42092

ENDF/B-VII.1

mo-94

42094

ENDF/B-VII.1

mo-95

42095

ENDF/B-VII.1

mo-96

42096

ENDF/B-VII.1

mo-97

42097

ENDF/B-VII.1

mo-98

42098

ENDF/B-VII.1

mo-99

42099

BLO approximation data

n-14

7014

BLO approximation data

n-15

7015

ENDF/B-VII.1

na-23

11023

ENDF/B-VII.1

nb-93

41093

ENDF/B-VI

nb-94

41094

BLO approximation data

nb-95

41095

ENDF/B-VII.1

nd-142

60142

BLO approximation data

nd-143

60143

ENDF/B-VII.1

nd-144

60144

BLO approximation data

nd-145

60145

ENDF/B-VII.1

nd-146

60146

ENDF/B-VII.1

nd-147

60147

BLO approximation data

nd-148

60148

ENDF/B-VII.1

nd-148

60148

BLO approximation data

nd-150

60150

BLO approximation data

ni-58

28058

ENDF/B-VII.1

ni-59

28059

BLO approximation data

ni-60

28060

ENDF/B-VII.1

ni-61

28061

ENDF/B-VI

ni-62

28062

ENDF/B-VI

ni-64

28064

ENDF/B-VI

np-234

93234

ENDF/B-VII.1

np-235

93235

ENDF/B-VII.1

np-236

93236

ENDF/B-VII.1

np-237

93237

ENDF/B-VII.1

\(\chi\) covariance JENDL-4.0

np-238

93238

ENDF/B-VII.1

np-239

93239

ENDF/B-VII.1

o-16

8016

ENDF/B-VII.1

o-17

8017

BLO approximation data

o-beo

5008016

ENDF/B-VII.1

Duplicate of o-16

o-uo2

1008016

ENDF/B-VII.1

Duplicate of o-16

p-31

15031

BLO approximation data

pa-229

91229

ENDF/B-VII.1

pa-230

91230

ENDF/B-VII.1

pa-231

91231

BLO approximation data

\(\chi\) covariance JENDL-4.0

pa-232

91232

ENDF/B-VII.1

pa-233

91233

BLO approximation data

\(\chi\) covariance JENDL-4.0

pb-204

82204

ENDF/B-VII.1

pb-206

82206

ENDF/B-VII.1

pb-207

82207

ENDF/B-VII.1

pb-208

82208

ENDF/B-VII.1

pd-102

46102

BLO approximation data

pd-104

46104

BLO approximation data

pd-105

46105

ENDF/B-VII.1

pd-106

46106

ENDF/B-VII.1

pd-107

46107

ENDF/B-VII.1

pd-108

46108

ENDF/B-VII.1

pd-110

46110

BLO approximation data

pm-147

61147

ENDF/B-VII.1

Thermal and resonance range uncertainty values from Mughabghab

pm-148

61148

BLO approximation data

pm-148m

1061148

BLO approximation data

pm-149

61149

BLO approximation data

pm-151

61151

BLO approximation data

pr-141

59141

ENDF/B-VII.1

pr-142

59142

BLO approximation data

pr-143

59143

BLO approximation data

pu-236

94236

ENDF/B-VII.1

pu-237

94237

ENDF/B-VII.1

pu-238

94238

ENDF/B-VII.1

pu-239

94239

ENDF/B-VII.2 prelim

pu-240

94240

ENDF/B-VII.1

pu-241

94241

ENDF/B-VII.1 \(\chi\) covariance JENDL-4.0

pu-242

94242

ENDF/B-VII.1

pu-243

94243

BLO approximation data

pu-244

94244

ENDF/B-VII.1

pu-246

94246

ENDF/B-VII.1

rb-85

37085

BLO approximation data

rb-86

37086

BLO approximation data

rb-87

37087

BLO approximation data

re-185

75185

ENDF/B-VI

re-187

75187

ENDF/B-VI

rh-103

45103

ENDF/B-VII.1

Uses ENDF/B-VII.1 data uncertainty in the thermal range for MT=102

rh-105

45105

BLO approximation data

ru-100

44100

BLO approximation data

ru-101

44101

ENDF/B-VII.1

ru-102

44102

ENDF/B-VII.1

ru-103

44103

ENDF/B-VII.1

ru-104

44104

ENDF/B-VII.1

ru-105

44105

BLO approximation data

ru-106

44106

ENDF/B-VII.1

ru-96

44096

BLO approximation data

ru-98

44098

BLO approximation data

ru-99

44099

BLO approximation data

s

16000

BLO approximation data

s-32

16032

BLO approximation data

s-33

16033

BLO approximation data

s-34

16034

BLO approximation data

s-36

16036

BLO approximation data

sb-121

51121

BLO approximation data

sb-123

51123

BLO approximation data

sb-124

51124

BLO approximation data

sb-125

51125

BLO approximation data

sb-126

51126

BLO approximation data

sc-45

21045

ENDF/B-VI

se-74

34074

BLO approximation data

se-76

34076

BLO approximation data

se-77

34077

BLO approximation data

se-78

34078

BLO approximation data

se-79

34079

BLO approximation data

se-80

34080

BLO approximation data

se-82

34082

BLO approximation data

si

14000

ENDF/B-VI

si-28

14028

ENDF/B-VII.1

si-29

14029

ENDF/B-VII.1

si-30

14030

ENDF/B-VII.1

si-28 in SiO2

14728

ENDF/B-VII.1

Duplicate of si-28

si-29 in SiO2

14729

ENDF/B-0VII.1

Duplicate of si-29

si-30 in SiO2

14730

ENDF/B-VII.1

Duplicate of si-30

sm-144

62144

BLO approximation data

sm-147

62147

BLO approximation data

sm-148

62148

BLO approximation data

sm-149

62149

ENDF/B-VII.1

Uses ENDF/B-VII.1 data uncertainty in the thermal range for MT=102

sm-149

62149

BLO approximation data

sm-150

62150

BLO approximation data

sm-151

62151

ENDF/B-VII.1

Uses ENDF/B-VII.1 data uncertainty in the thermal range for MT=102

sm-152

62152

ENDF/B-VII.1

sm-153

62153

BLO approximation data

sm-154

62154

BLO approximation data

sn-112

50112

BLO approximation data

sn-113

50113

BLO approximation data

sn-114

50114

BLO approximation data

sn-115

50115

BLO approximation data

sn-116

50116

BLO approximation data

sn-117

50117

BLO approximation data

sn-118

50118

BLO approximation data

sn-119

50119

BLO approximation data

sn-120

50120

BLO approximation data

sn-122

50122

BLO approximation data

sn-123

50123

BLO approximation data

sn-124

50124

BLO approximation data

sn-125

50125

BLO approximation data

sn-126

50126

BLO approximation data

sr-84

38084

BLO approximation data

sr-86

38086

BLO approximation data

sr-87

38087

BLO approximation data

sr-88

38088

BLO approximation data

sr-89

38089

BLO approximation data

sr-90

38090

BLO approximation data

ta-181

73181

BLO approximation data

ta-182

73182

BLO approximation data

tb-159

65159

BLO approximation data

tb-160

65160

BLO approximation data

tc-99

43099

ENDF/B-VII.1

te-120

52120

BLO approximation data

te-122

52122

BLO approximation data

te-123

52123

BLO approximation data

te-124

52124

BLO approximation data

te-125

52125

BLO approximation data

te-126

52126

BLO approximation data

te-127m

1052127

BLO approximation data

te-128

52128

BLO approximation data

te-129m

1052129

BLO approximation data

te-130

52130

BLO approximation data

te-132

52132

BLO approximation data

th-227

90227

ENDF/B-VII.1

th-228

90228

ENDF/B-VII.1

th-229

90229

ENDF/B-VII.1

th-230

90230

ENDF/B-VII.1

th-231

90231

ENDF/B-VII.1

th-232

90232

ENDF/B-VII.1

\(\chi\) covariance JENDL-4.0

th-233

90233

ENDF/B-VII.1

th-234

90234

ENDF/B-VII.1

ti

22000

BLO approximation data

ti-46

22046

ENDF/B-VII.1

ti-47

22047

ENDF/B-VII.1

ti-48

22048

ENDF/B-VII.1

ti-49

22049

ENDF/B-VII.1

ti-50

22050

ENDF/B-VII.1

tl-203

81203

ENDF/B-VII.1

tl-205

81205

ENDF/B-VII.1

tm-169

69169

ENDF/B-VII.1

tm-170

69170

ENDF/B-VII.1

u-230

92230

ENDF/B-VII.1

u-231

92231

ENDF/B-VII.1

u-232

92232

ENDF/B-VII.1

u-233

92233

ENDF/B-VII.1

\(\chi\) covariance JENDL-4.0

u-234

92234

ENDF/B-VII.1

u-235

92235

ENDF/B-VII.2 prelim

u-236

92236

ENDF/B-VII.1

u-237

92237

BLO approximation data

u-238

92238

ENDF/B-VII.1

u-239

92239

BLO approximation data

u-240

92240

BLO approximation data

u-241

92241

BLO approximation data

u-uo2

1092235

ENDF/B-VII.1

Duplicate of u-235

v

23000

BLO approximation data

v-50

23050

BLO approximation data

Duplicate of v

v-51

23051

BLO approximation data

Duplicate of v

w

74000

BLO approximation data

w-180

74180

ENDF/B-VII.1

w-182

74182

ENDF/B-VII.1

w-183

74183

ENDF/B-VII.1

w-184

74184

ENDF/B-VII.1

w-186

74186

ENDF/B-VII.1

xe-123

54123

BLO approximation data

xe-124

54124

BLO approximation data

xe-126

54126

BLO approximation data

xe-128

54128

BLO approximation data

xe-129

54129

BLO approximation data

xe-130

54130

BLO approximation data

xe-131

54131

ENDF/B-VII.1

xe-132

54132

ENDF/B-VII.1

xe-133

54133

BLO approximation data

xe-134

54134

ENDF/B-VII.1

xe-135

54135

BLO approximation data

xe-136

54136

BLO approximation data

y-89

39089

ENDF/B-VII.1

y-90

39090

BLO approximation data

y-91

39091

BLO approximation data

zr

40000

BLO approximation data

zr-90

40090

ENDF/B-VII.1

zr-91

40091

ENDF/B-VII.1

zr-92

40092

ENDF/B-VII.1

zr-93

40093

ENDF/B-VII.1

zr-94

40094

ENDF/B-VII.1

zr-95

40095

ENDF/B-VII.1

zr-96

40096

ENDF/B-VII.1

zr-90-zr5h8

1040090

ENDF/B-VII.1

Duplicate of zr-90

zr-91-zr5h8

1040091

ENDF/B-VII.1

Duplicate of zr-91

zr-92-zr5h8

1040092

ENDF/B-VII.1

Duplicate of zr-92

zr-93-zr5h8

1040093

ENDF/B-VII.1

Duplicate of zr-93

zr-94-zr5h8

1040094

ENDF/B-VII.1

Duplicate of zr-94

zr-95-zr5h8

1040095

ENDF/B-VII.1

Duplicate of zr-95

zr-96-zr5h8

1040096

ENDF/B-VII.1

Duplicate of zr-96

Table 10.3.2 Covariance data with cross-correlations between nuclide reactions.

Nuclide 1

Reaction 1

Nuclide 2

Reaction 2

239Pu

Fission

6Li

Triton production

239Pu

Fission

197Au

Capture

239Pu

Fission

235U

Fission

239Pu

Fission

238U

Fission

235U

Fission

197Au

Capture

235U

Fission

6Li

Triton production

238U

Capture

197Au

Capture

238U

Capture

235U

Fission

10.3.5. SCALE 6.1 44-group covariance library

The older 44-group covariance library distributed with SCALE 6.0 and SCALE 6.1 is included with this distribution for backwards compatibility. The 44-group covariance library provides uncertainty data for a total of 401 materials, including some duplication for materials with multiple thermal scattering kernels. However, the 44-group library was created prior to the official release of ENDF/B-VII.1. Therefore, it is recommended that the 56- or 252-group covariances be used rather than the 44-group. As discussed in Sect. 10.3.1, it is assumed that covariances taken from one data evaluation such as ENDF/B-VI or JENDL-3.3 can also be applied to other evaluations of the same data, such as ENDF/B-VII. If this is done judiciously for cases in which the nuclear data evaluations are similar, then the covariances taken from one source should be a reasonable representation of uncertainties for the other evaluations. Among the materials in the SCALE 44-group library with covariances taken from high-fidelity nuclear data evaluations are the following:

a) ENDF/B-VII evaluations (includes both VII.0 and pre-release covariances proposed for VII.1, but no official ENDF/B-VII.1):

Au, 209Bi, 59Co, 152,154,155,156Gd, 191,193I, 7Li, 23Na, 93Nb, 58Ni, 99Tc,232Th, 48Ti, 239Pu, 233,235,238U,V

  1. ENDF/B-VI evaluations:

Al, 241Am, 10B, 12C, 50,52,53,54Cr, 63,65Cu, 54,56,57Fe, In, 55Mn, 60,61,62,64Ni, 206,207,208Pb, 242Pu, 28,29Si

  1. JENDL-3.3 evaluations:

11B, 1H, 16O, 240,241Pu

Two modifications were also made to the ENDF/B-VII evaluated nubar covariances. These nubar uncertainties are believed to be more realistic. The ENDF/B-VII.0 235U thermal nubar uncertainty of 0.71% was revised to the JENDL-3.3 value of 0.31%. In addition, the thermal nubar certainty in the pre-released ENDF/B-VII.1 233U evaluation was modified to the value in a recent ORNL data evaluation [COVLIBLWRD08]. This ORNL 233U cross section evaluation also provided the thermal and resonance cross sections for the prereleased ENDF/B-VII.1 data. The ENDF/B-VII.1 pre-release nubar data for 239Pu was incomplete when the 44-group covariance library was generated, so 239Pu nubar data are included from ENDF/B-V, the most current data available at that time. This value is much higher than the current estimated uncertainty in 239Pu nubar. The basic ENDF/B uncertainty files that were changed are described in Table 10.3.3.

Several modifications were also made to the uncertainties obtained from the BLO data. The BLO thermal uncertainties for 1H capture and elastic and for 16O elastic were modified to the JENDL-3.3 values of 0.5% and 0.1%, respectively. Similarly, the uncertainty in the 10B (n,alpha) thermal cross section was modified to the ENDF/B-VI value of about 0.2%, since this is more consistent with the Mughabghab integral uncertainty. The uncertainty in the 149Sm resonance capture integral is not provided in the 2006 edition of Mughabghab’s text; therefore it was set to the value of 5.7% which was obtained from an earlier tabulation by Mughabghab [COVLIBMug03].

Table 10.3.3 Summary of changes made to covariance evaluations for the 44-group library.

ENDF/B-VII.1 pre-release

239Pu

Data were incomplete at time of library generation, so ENDF/B-V data were used for nubar.

ENDF/B-VII

235U

Thermal nubar modified to JENDL-3.3 value

ENDF/B-VII

233U

Thermal nubar modified to value from ORNL internal evaluation

ENDF/B-VI

241Am

Thermal uncertainties were added to total cross section (set equal to capture uncertainties)

ENDF/B-VI

28Si, 29Si, 30Si, 206Pb, 57Fe

In elastic scatter uncertainty, corrected cross reference to MT=102 from original value of MT=1.02

ENDF/B-VI

208Pb, 207Pb

Removed MT=3 due to inconsistency with other MT values, resulting in very large uncertainty predictions

At the time of the preparation of the 44-group covariance library, ENDF/B did not provide fission spectra uncertainty estimates. The methodology used to construct these data for the 44-group covariance library is described in Broadhead and Wagschal [COVLIBBW04]. In this approach, the fission spectrum is represented as either a Watt or Maxwellian distribution. These energy distributions are widely used to represent fission spectra and have been commonly employed in many ENDF/B evaluations. For example, Watt and Maxwellian expressions were used almost exclusively to describe fission spectra in ENDF/B-V and also for many ENDF/B-VI evaluations. More recent evaluations for some important fissionable nuclides have replaced the simple Watt and Maxwellian analytical expressions by distributions such as the Madland-Nix spectrum obtained from more phenomenological nuclear fission models. However, it is assumed here that uncertainties based on an appropriate Watt or Maxwellian representation of the fission spectrum can be transferred to the actual fission spectra contained in the different multigroup cross section libraries.

The methodology in Broadhead and Wagschal [COVLIBBW04] determines energy-dependent covariances from uncertainties and correlations in the a and b parameters for the Watt spectrum or the T parameter for a Maxwellian spectrum, appearing the analytical expressions given below:

Watt Spectrum: \(\chi(\mathrm{E})=\frac{\mathrm{e}^{-\mathrm{E} / \mathrm{a}}}{\mathrm{I}} \sinh (\sqrt{\mathrm{bE}})\)

Maxwellian Spectrum: \(\chi(\mathrm{E})=\frac{\sqrt{\mathrm{E}} \mathrm{e}^{-\mathrm{E} / \mathrm{T}}}{\mathrm{I}}\)

In these expressions, the parameter “I” is the normalization factor required to normalize the integrated spectrum to unity. The value of “I” is fixed by the values of the other parameters. Due to the normalization constraint, the fission spectrum covariance includes anti-correlations. The assumed fission spectra parameters and uncertainties are given in Maerker, Marable, and Wagschal 1980 [COVLIBMMW80] and in Howerton and Doyas 1971 [COVLIBHD71].

Table 10.3.4 shows that fission spectra covariances are not provided for all fissionable materials in the SCALE multigroup cross sections. Table 10.3.5 lists the fissionable nuclides without fission spectra covariances on the 44-group covariance library.

Table 10.3.4 Source of fission spectrum parameters and uncertainties

Watt spectrum

a or T

b

Source of parameters

\(\sigma_a\) or \(\sigma_T\) (%)

\(\sigma_b\)

(%)

Source of uncertainty

235U

0.988

2.249

ENDF/B-V

1.2

5.9

TANS16

238U

0.881

3.401

ENDF/B-V

1.2

5.9

TANS16

233U

0.977

2.546

ENDF/B-V

1.2

5.9

TANS16

239Pu

0.966

2.842

ENDF/B-V

1.2

5.9

TANS16

232Th

1.0888

1.6871

ENDF/B-V

1.2

5.9

TANS16

252Cf

1.025

2.926

ENDF/B-V

1.2

5.9

TANS16

Maxwellian Spectrum

238Pu

1.330

-

ENDF/B-V

3.01

-

NSE17

240Pu

1.346

-

ENDF/B-V

2.97

-

NSE17

241Pu

1.3597

-

ENDF/B-V

2.50

-

NSE17

242Pu

1.337

-

ENDF/B-V

5.24

-

NSE17

Table 10.3.5 Fissionable nuclides with missing fission spectrum uncertainty data in covariance library.

241Am

244Cm

238Pu

242Am

245Cm

243Pu

243Am

246Cm

244Pu

249Bk

247Cm

230Th

249Cf

248Cm

232U

250Cf

237Np

234U

251Cf

238Np

236U

253Cf

239Np

237U

242Cm

231Pa

243Cm

233Pa

Table 10.3.6 describes the contents of the library using the following nomenclature:

  1. ENDF/B-VII.0: evaluated covariance data released with ENDF/B-VII.0

  2. ENDF/B-VII-p: recently evaluated data proposed for future release of ENDF/B-VII.1

  3. ENDF/B-VI: evaluated covariance data released with ENDF/B-VI

  4. JENDL-3.3: evaluated covariance data in JENDL-3.3

  5. BLO approximate data: lo-fi covariances from BLO project

  6. BLO LANL evaluation: LANL R-matrix evaluation from BLO project

  7. SG-26: approximate covariances from WPEC Subgroup-26

Table 10.3.6 Contents of SCALE 6.1 44-group covariance library.

SCALE name

Data source

Comments

ac-225

BLO approximate data

ac-226

BLO approximate data

ac-227

BLO approximate data

ag-107

BLO approximate data

ag-109

BLO approximate data

ag-110m

BLO approximate data

ag-111

BLO approximate data

al-27

ENDF/B-VI

am-241

ENDF/B-VI

MT=452 added corrections for total and elastic)

am-242

SG-26

Thermal uncertainty replaced by Mughabghab value

am-242m

SG-26

Thermal uncertainty replaced by Mughabghab value

am-243

BLO approximate data

am-244

BLO approximate data

am-244m

BLO approximate data

ar-36

BLO approximate data

ar-38

BLO approximate data

ar-40

BLO approximate data

as-74

BLO approximate data

as-75

BLO approximate data

au-197

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

b-10

BLO LANL evaluation +ENDF/B-VI

LANL high-fidelity covariance, with ENDF/B-VI for thermal

b-11

JENDL 3.3

ba-130

BLO approximate data

ba-132

BLO approximate data

ba-133

BLO approximate data

ba-135

BLO approximate data

ba-136

BLO approximate data

ba-137

BLO approximate data

ba-138

BLO approximate data

ba-140

BLO approximate data

be-7

BLO approximate data

be-9

BLO approximate data

Bebound

BLO approximate data

Duplicate of 9Be

bi-209

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

bk-249

BLO approximate data

bk-250

BLO approximate data

br-79

BLO approximate data

br-81

BLO approximate data

C

ENDF/B-VI

C-graphite

ENDF/B-VI

Duplicate of carbon

Ca

BLO approximate data

ca-40

BLO approximate data

ca-42

BLO approximate data

ca-43

BLO approximate data

ca-44

BLO approximate data

ca-46

BLO approximate data

ca-48

BLO approximate data

Cd

BLO approximate data

cd-106

BLO approximate data

cd-108

BLO approximate data

cd-110

BLO approximate data

cd-111

BLO approximate data

cd-112

BLO approximate data

cd-113

BLO approximate data

cd-114

BLO approximate data

cd-115m

BLO approximate data

cd-116

BLO approximate data

cd-136

BLO approximate data

cd-138

BLO approximate data

cd-139

BLO approximate data

cd-140

BLO approximate data

cd-141

BLO approximate data

cd-142

BLO approximate data

ce-143

BLO approximate data

ce-144

BLO approximate data

cf-249

BLO approximate data

cf-250

BLO approximate data

cf-251

BLO approximate data

cf-252

BLO approximate data

cf-253

BLO approximate data

cf-254

BLO approximate data

Cl

BLO approximate data

cl-35

BLO approximate data

cl-37

BLO approximate data

cm-241

BLO approximate data

Thermal uncertainty

cm-242

SG-26

Mughabghab value

cm-243

SG-26

Thermal uncertainty replaced by Mughabghab value

cm-244

SG-26

Thermal uncertainty replaced by Mughabghab value

cm-245

SG-26

Thermal uncertainty replaced by Mughabghab value

cm-246

BLO approximate data

cm-247

BLO approximate data

cm-248

BLO approximate data

cm-249

BLO approximate data

cm-250

BLO approximate data

co-58

co-58m

co-59

BLO approximate data

BLO approximate data

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

cr-50

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

cr-52

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

cr-53

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

cr-54

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

cs-133

BLO approximate data

cs-134

BLO approximate data

cs-135

BLO approximate data

cs-136

BLO approximate data

cs-137

BLO approximate data

cu-63

ENDF/B-VI

cu-65

ENDF/B-VI

dy-156

BLO approximate data

dy-158

BLO approximate data

dy-160

BLO approximate data

dy-161

BLO approximate data

dy-162

BLO approximate data

dy-163

BLO approximate data

dy-164

BLO approximate data

er-162

BLO approximate data

er-164

BLO approximate data

er-166

BLO approximate data

er-167

BLO approximate data

er-168

BLO approximate data

er-170

BLO approximate data

es-253

BLO approximate data

es-254

BLO approximate data

es-255

BLO approximate data

eu-151

BLO approximate data

eu-152

BLO approximate data

eu-153

BLO approximate data

eu-154

BLO approximate data

eu-155

eu-156

eu-157

BLO approximate data BLO approximate data BLO approximate data

f-19

BLO approximate data

fe-54

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

fe-56

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

fe-57

ENDF/B-VI

Error in file corrected LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

fe-58

fm-255

ENDF/B-VI

BLO approximate data

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results. New material not in previous

SCALE 5.1 covariance libraries.

Ga

ga-69

ga-71

BLO approximate data

BLO approximate data

BLO approximate data

gd-152

gd-153

ENDF/B-VII.0

BLO approximate data

gd-154

ENDF/B-VII.0

gd-155

ENDF/B-VII.0

gd-156

ENDF/B-VII.0

gd-157

ENDF/B-VII.0

gd-158

ENDF/B-VII.0

gd-160

ENDF/B-VII.0

ge-70

BLO approximate data

ge-72

BLO approximate data

ge-73

BLO approximate data

ge-74

BLO approximate data

ge-76

BLO approximate data

h-1

BLO LANL evaluation +JENDL 3.3

LANL covariance above 5 keV; JENDL values below 5 keV

h-ZrH

BLO LANL evaluation +JENDL 3.

Duplicate of 1H

h-poly

BLO LANL evaluation +JENDL 3.

Duplicate of 1H

Hfreegas

BLO LANL evaluation +JENDL 3.

Duplicate of 1H

h-2

BLO approximate data

Dfreegas

BLO approximate data

Duplicate of 2H

h-3

BLO approximate data

he-3

BLO approximate data

he-4

BLO approximate data

Hf

BLO approximate data

hf-174

BLO approximate data

hf-176

BLO approximate data

fh-177

BLO approximate data

hf-178

BLO approximate data

hf-179

BLO approximate data

hf-180

BLO approximate data

hg-196

BLO approximate data

hg-198

BLO approximate data

hg-199

BLO approximate data

hg-200

BLO approximate data

hg-201

BLO approximate data

hg-202

BLO approximate data

hg-204

BLO approximate data

ho-165

BLO approximate data

i-127

BLO approximate data

i-129

BLO approximate data

i-130

BLO approximate data

i-131

BLO approximate data

i-135

BLO approximate data

In

ENDF/B-VI

in-113

in-115

BLO approximate data

BLO approximate data

ir-191

ENDF/B-VII.0

ir-193

ENDF/B-VII.0

K

BLO approximate data

k-39

BLO approximate data

k-40

BLO approximate data

k-41

BLO approximate data

kr-78

BLO approximate data

kr-80

BLO approximate data

kr-82

BLO approximate data

kr-83

BLO approximate data

kr-84

BLO approximate data

kr-85

BLO approximate data

kr-86

BLO approximate data

la-138

la-139

BLO approximate data BLO approximate data

la-140

BLO approximate data

li-6

BLO-LANL evaluation

li-7

ENDF/B-VII.0

lu-175

BLO approximate data

lu-176

BLO approximate data

Mg

BLO approximate data

mg-24

BLO approximate data

mg-25

BLO approximate data

mg-26

BLO approximate data

mn-55

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

Mo

BLO approximate data

mo-92

BLO approximate data

mo-94

BLO approximate data

mo-95

BLO approximate data

mo-96

BLO approximate data

mo-97

BLO approximate data

mo-98

mo-99

mo-100

BLO approximate data BLO approximate data

BLO approximate data

n-14

BLO approximate data

n-15

BLO approximate data

na-23

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

nb-93

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

nb-94

BLO approximate data

nb-95

BLO approximate data

nd-142

BLO approximate data

nd-143

BLO approximate data

nd-144

BLO approximate data

nd-145

BLO approximate data

nd-146

BLO approximate data

nd-147

BLO approximate data

nd-148

BLO approximate data

nd-150

BLO approximate data

ni-58

ni-59

ENDF/B-VII-p

BLO approximate data

Pre-released evaluation proposed for ENDF/B-VII.1

ni-60

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

ni-61

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

ni-62

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

ni-64

ENDF/B-VI

LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

np-235

np-236

np-237

BLO approximate data

BLO approximate data

SG-26

Thermal uncertainty replaced by Mughabghab value

np-238

BLO approximate data

np-239

BLO approximate data

o-16

JENDL 3.3+BLO

BLO covariances from LANL used above 5 keV

o-17

BLO approximate data

p-31

BLO approximate data

pa-231

pa-232

BLO approximate data

BLO approximate data

pa-233

BLO approximate data

pb-204

pb-206

BLO approximate data ENDF/B-VI

Error in file corrected

pb-207

ENDF/B-VI

MT=3 removed, Error in file corrected

bp-208

ENDF/B-VI

MT=3 removed, Error in file corrected

pd-102

BLO approximate data

pd-104

BLO approximate data

pd-105

BLO approximate data

pd-106

BLO approximate data

pd-107

BLO approximate data

pd-108

BLO approximate data

pd-110

BLO approximate data

pm-147

BLO approximate data

pm-148

BLO approximate data

pm-148m

BLO approximate data

pm-149

BLO approximate data

pm-151

BLO approximate data

pr-141

BLO approximate data

pr-142

BLO approximate data

pr-143

BLO approximate data

pu-236

pu-237

pu-238

BLO approximate data

BLO approximate data

SG-26

Thermal uncertainty replaced by Mughabghab value

pu-239

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1; nubar data from ENDF/B-V

Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide Table 10.3.2

pu-240

JENDL 3.3

Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (Table 10.3.2

pu-241

JENDL 3.3

Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (Table 10.3.2)

pu-242

ENDF/B-VI

pu-243

BLO approximate data

pu-244

BLO approximate data

pu-246

BLO approximate data

rb-85

BLO approximate data

rb-86

BLO approximate data

rb-87

BLO approximate data

re-185

ENDF/B-VI

MT=2 added from Mughabghab. LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

re-187

ENDF/B-VI

MT=2 added from Mughabghab. LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

rh-103

BLO approximate data

rh-105

BLO approximate data

ru-96

BLO approximate data

ru-98

BLO approximate data

ru-103

BLO approximate data

ru-99

BLO approximate data

ru-100

BLO approximate data

ru-101

BLO approximate data

ru-102

BLO approximate data

ru-104

BLO approximate data

ru-105

BLO approximate data

ru-106

BLO approximate data

S

BLO approximate data

s-32

BLO approximate data

s-33

BLO approximate data

s-34

BLO approximate data

s-36

BLO approximate data

sb-123

BLO approximate data

sb-124

BLO approximate data

sb-125

BLO approximate data

sb-126

BLO approximate data

sc-45

ENDF/B-VI

se-74

BLO approximate data

se-76

BLO approximate data

se-77

BLO approximate data

se-78

se-79

BLO approximate data BLO approximate data

se-80

BLO approximate data

se-82

BLO approximate data

Si

ENDF/B-VI

si-28

ENDF/B-VI

Error in file corrected LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

si-29

ENDF/B-VI

Error in file corrected LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

si-30

ENDF/B-VI

Error in file corrected LB=8 representation caused problematic representation of cross section uncertainty due to use of fine energy group structure. Tests were performed to determine how to handle this problem. LB=8 data were removed in the final results.

sm-144

BLO approximate data

sm-147

BLO approximate data

sm-148

BLO approximate data

sm-149

BLO approximate data

Resonance range uncertainty from Kawano 2008

sm-150

BLO approximate data

sm-151

BLO approximate data

sm-152

BLO approximate data

sm-153

BLO approximate data

sm-154

BLO approximate data

sn-112

BLO approximate data

sn-113

BLO approximate data

sn-114

BLO approximate data

sn-115

BLO approximate data

sn-116

BLO approximate data

sn-117

BLO approximate data

sn-118

BLO approximate data

sn-119

BLO approximate data

sn-120

BLO approximate data

sn-122

BLO approximate data

sn-123

BLO approximate data

sn-124

BLO approximate data

sn-125

BLO approximate data

sr-84

BLO approximate data

sr-86

BLO approximate data

sr-87

BLO approximate data

sr-88

BLO approximate data

sr-89

BLO approximate data

sr-90

BLO approximate data

ta-181

BLO approximate data

ta-182

BLO approximate data

tb-159

BLO approximate data

tb-160

BLO approximate data

tc-99

ENDF/B-VII.0

te-120

BLO approximate data

te-122

BLO approximate data

te-123

BLO approximate data

te-124

BLO approximate data

te-125

BLO approximate data

te-126

BLO approximate data

te-127m

BLO approximate data

te-128

BLO approximate data

te-129m

BLO approximate data

te-130

BLO approximate data

th-227

BLO approximate data

th-228

BLO approximate data

th-229

BLO approximate data

th-230

BLO approximate data

th-232

th-233

th-234

Ti

ti-46

ti-47

ti-48

ENDF/B-VII.0

BLO approximate data

BLO approximate data

BLO approximate data

BLO approximate data

BLO approximate data

ENDF/B-VII-p

Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (Table 10.3.2)

Pre-released evaluation proposed for ENDF/B-VII.1

ti-49

BLO approximate data

ti-50

BLO approximate data

u-232

BLO approximate data

u-233

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1; nubar uncertainty from Ref. 14Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (

Table 10.3.2).

u-234

SG-26

Thermal uncertainty replaced by Mughabghab value

u-235

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1; nubar uncertainty from JENDL-3.1 Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (Table 10.3.2).

u-236

SG-26

Thermal uncertainty replaced by Mughabghab value

u-237

BLO approximate data

u-238

u-239

u-240

u-241

ENDF/B-VII-p

BLO approximate data

BLO approximate data

BLO approximate data

Pre-released evaluation proposed for ENDF/B-VII.1 Cross nuclide-to-nuclide matrices present; covariances due to fission cross sections / nubar for each nuclide (Table 10.3.2).

V

ENDF/B-VII-p

Pre-released evaluation proposed for ENDF/B-VII.1

W

BLO approximate data

w-182

BLO approximate data

w-183

BLO approximate data

w-184

BLO approximate data

w-186

BLO approximate data

xe-123

BLO approximate data

xe-124

BLO approximate data

xe-126

BLO approximate data

xe-128

BLO approximate data

xe-129

BLO approximate data

xe-130

BLO approximate data

xe-131

BLO approximate data

xe-132

BLO approximate data

xe-134

BLO approximate data

xe-135

BLO approximate data

xe-136

BLO approximate data

y-89

ENDF/B-VI

y-90

BLO approximate data

y-91

BLO approximate data

Zr

BLO approximate data

zr-90

BLO approximate data

zr-91

BLO approximate data

zr-92

BLO approximate data

zr-93

BLO approximate data

zr-94

BLO approximate data

zr-95

BLO approximate data

zr-96

BLO approximate data

Table 10.3.7 Covariance data with cross correlations between nuclide reactions.

Nuclide 1

Reaction 1

Nuclide 2

Reaction 2

240Pu

Fission

239Pu

Fission

240Pu

Fission

233U

Fission

240Pu

Fission

238U

Fission

241Pu

Fission

239Pu

Fission

241Pu

Fission

240Pu

Fission

241Pu

Fission

233U

Fission

241Pu

Fission

235U

Fission

241Pu

Fission

238U

Fission

235U

Fission

240Pu

Fission

References

COVLIBBW04(1,2)

Bryan L. Broadhead and J. J. Wagschal. The Fission Spectrum Uncertainty. PHYSOR 2004–The Physics of Fuel Cycles and Advanced Nuclear Systems: Global Developments, pages 25–29, 2004.

COVLIBCHO+11

M.B. Chadwick, M. Herman, P. Obložinský, M.E. Dunn, Y. Danon, A.C. Kahler, D.L. Smith, B. Pritychenko, G. Arbanas, R. Arcilla, R. Brewer, D.A. Brown, R. Capote, A.D. Carlson, Y.S. Cho, H. Derrien, K. Guber, G.M. Hale, S. Hoblit, S. Holloway, T.D. Johnson, T. Kawano, B.C. Kiedrowski, H. Kim, S. Kunieda, N.M. Larson, L. Leal, J.P. Lestone, R.C. Little, E.A. McCutchan, R.E. MacFarlane, M. MacInnes, C.M. Mattoon, R.D. McKnight, S.F. Mughabghab, G.P.A. Nobre, G. Palmiotti, A. Palumbo, M.T. Pigni, V.G. Pronyaev, R.O. Sayer, A.A. Sonzogni, N.C. Summers, P. Talou, I.J. Thompson, A. Trkov, R.L. Vogt, S.C. van der Marck, A. Wallner, M.C. White, D. Wiarda, and P.G. Young. ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data. Nuclear Data Sheets, 112(12):2887–2996, 2011. URL: https://www.sciencedirect.com/science/article/pii/S009037521100113X, doi:https://doi.org/10.1016/j.nds.2011.11.002.

COVLIBHal08

Gerald Hale. Covariances from light-element r-martix analyses. Technical Report, Los Alamos National Laboratory, Los Alamos, NM (USA), 2008.

COVLIBHD71

R. J. Howerton and R. J. Doyas. Fission temperatures as a function of the average number of neutrons from fission. Nuclear Science and Engineering, 46(3):414–416, 1971. Publisher: Taylor & Francis.

COVLIBKTY+08

T. Kawano, P. Talou, P. G. Young, G. Hale, M. B. Chadwick, and R. C. Little. Evaluation of covariances for actinides and light elements at LANL. Nuclear Data Sheets, 109(12):2817–2821, 2008.

COVLIBLLD+06

N. M. Larson, L. C. Leal, H. Derrien, G. Arbanas, R. O. Sayer, and D. Wiarda. A systematic description of the generation of covariance matrices. In PHYSOR-2006: ANS Topical Meeting on Reactor Physics, 10–14. 2006.

COVLIBLWRD08

Luiz C. Leal, D. Wiarda, Bradley T. Rearden, and Herve Derrien. 233 U Cross-Section and Covariance Data Update for SCALE 5.1 Libraries. ORNL/TM-2007/115, Oak Ridge National Laboratory, Oak Ridge, Tenn, 2008.

COVLIBLKH+08(1,2)

R. C. Little, T. Kawano, G. D. Hale, M. T. Pigni, M. Herman, P. Obložinsky, M. L. Williams, M. E. Dunn, G. Arbanas, and D. Wiarda. Low-fidelity Covariance Project. Nuclear Data Sheets, 109(12):2828–2833, 2008. Publisher: Elsevier.

COVLIBMMW80

R. E. Maerker, J. H. Marable, and J. J. Wagschal. Estimation of the uncertainties in the ENDF/BV Uranium 235 fission spectrum. In Transactions of the American Nuclear Society, volume 35. 1980.

COVLIBMug03(1,2)

S. F. Mughabghab. Thermal neutron capture cross sections resonance integrals and g-factors. International Atomic Energy Agency, 2003.

COVLIBMug06(1,2)

Said F. Mughabghab. Atlas of Neutron Resonances: Resonance Parameters and Thermal Cross Sections. Z= 1-100. Elsevier, 2006.

COVLIBPHO09

M. T. Pigni, M. Herman, and P. Obložinsky. Extensive Set of Cross-Section Covariance Estimates in the Fast Neutron Region. Nuclear science and engineering, 162(1):25–40, 2009. Publisher: Taylor & Francis.

COVLIBRHOM07

D. Rochman, M. Herman, P. Oblozinsky, and S. F. Mughabghab. Preliminary cross-section covariances for WPEC Subgroup 26. Technical Report BNL-77407-2007-IR, Brookhaven National Laboratory, Upton, NY (USA), 2007.

COVLIBWD06

D. Wiarda and M. E. Dunn. PUFF-IV: A Code for Processing ENDF Uncertainty Data into Multigroup Covariance Matrices. Technical Report ORNL/TM-2006/147, Oak Ridge National Laboratory, Oak Ridge, TN (USA), 10 2006.

COVLIBWALD08

Dorothea Wiarda, Goran Arbanas, L. Leal, and Michael E. Dunn. Recent advances with the AMPX covariance processing capabilities in PUFF-IV. Nuclear Data Sheets, 109(12):2791–2795, 2008. Publisher: Elsevier.

COVLIBWBDR07

Mark L. Williams, Bryan L. Broadhead, Michael E. Dunn, and Bradley T. Rearden. Approximate Techniques for Representing Nuclear Data Uncertainties. In Eighth International Topical Meeting on Nuclear Applications and Utilization of Accelerators (AccApp'07)," Pocatello, ID (July 30-Aug. 2, 2007). 7 2007.

COVLIBWIMR14

Mark L. Williams, Germina Ilas, William J. Marshall, and Bradley T. Rearden. Applications of nuclear data covariances to criticality safety and spent fuel characterization. Nuclear Data Sheets, 118:341–345, 2014.

COVLIBWR08(1,2,3,4,5)

Mark L. Williams and Bradley T. Rearden. SCALE-6 Sensitivity/uncertainty methods and covariance data. Nuclear Data Sheets, 109(12):2796–2800, 2008.